Famed for his roles in dozens of movies, including "Jewel Thief" and "Guide," the veteran actor, director and producer was working up to the last minute, with a new script in the works.
Anand lived and died on "his own terms," his nephew and renowned film director Shekhar Kapur said in a posting on Twitter. "He was working one minute. Sat down and smiled. And was gone the next. So much to learn."
Anand died of a heart attack Saturday night in a hotel in London, where he had gone recently for a medical checkup, the family said.
Born on Sept. 26, 1923, as the son of a Punjab lawyer, Anand studied English literature and law, eventually moving in his early 20s to India's film capital of Mumbai, then called Bombay, where he pursued acting.
Known for his good looks, melodious voice and success in romantic leads, Anand was considered a superstar within just a few years of his 1946 screen debut in the Hindi-language film "Hum Ek Hain."
Anand also began producing in 1949, and made his directorial debut in 1971 with the popular hippie cult film "Hare Rama Hare Krishna." Never giving up the career, Anand released his latest film, "Chargesheet," just a few months ago and was reportedly working on another script when he died.